Abstract

We observed for the first time a strong angle-independent modification of spontaneous emission spectra from laser dyes in photonic crystals, made of inverse opals in titania. Comparison with spectra from such crystals with much smaller lattice spacing, for which emission is in the long wavelength limit, reveals inhibition of emission up to a factor ∼5 over a large bandwidth of 13% of the first order Bragg resonance frequency. The center frequency and bandwidth of the inhibition agree with calculated total density of states, while the measured inhibition of vacuum fluctuations is much larger. Because of the specific location of the dye molecules, we likely probe the strongly modulated local photonic density of states.

URL

https://doi.org/10.1103/PhysRevLett.88.143903

Authors

A. F. Koenderink, L. Bechger, H. P. Schriemer, A. Lagendijk, and W. L. Vos

Year of publication

2002

Date published

03/2002

Journal

Phys. Rev. Lett.

Volume

88

Pages

143903: 1-4

DOI number

10.1103/PhysRevLett.88.143903

Keywords

3D photonic band gap crystals, inhibition, LDOS, Local density of optical states, spontaneous emission